TUNABLE DIODE LASER SPECTROSCOPY OF $CH_{3}F$ IN AN EQUILIBRIUM CELL MAINTAINED AT 7.5 KELVINS

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1994

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Ohio State University

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We report the infrared measurement of rotational and translational temperatures for $CH_{3}F$ in the gas phase with a temperature of 16 Kelvins. This is accomplished by extending the collisional cooling technique originally developed for the microwave spectral $region^{1}$ to the infrared. We measured an RQ(J,0) feature centered at approximately 1475 wavenumbers (in $cm^{-1}$) in the V2 and V5 bands of $CH_{3}F$. The rotational temperature was determined by measuring relative intensities of low J transitions and comparing these results to those predicted by the rotational partition function. We utilized measurements of the absorption line width to calculate the translational temperature.

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1. D.R. Willey, R.L. Crownover, D.N. Bittner and F.C. De Lucia, J. Chem. Phys. 89, 1923 (1988).
Author Institution: Department of Physics, Allegheny College; Department of Physics and Astronomy, Franklin and Marshall College

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