INTRAMOLECULAR STRAIN CONSTANTS: PYRAMIDAL $XY_{3}$ MOLECULES

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Date

1956

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Ohio State University

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Abstract

The potential function ${V}=\Sigma_{all bonds}\qquad {k}_{i}({d}_{i}-{D}_{i}^{0})^{2}+\Sigma_{all angles}\qquad {k}_{a}(a_{j}-{A}_{j}^{0})^{2}$, where $D^{0}_{i}$ and $A^{0}_{j}$ are the ""Strain free"" values of bond length and bond angle respectively, has been extended to $NH_{3}$-type molecules. Improved mathematics are described. Sufficient equations exist to determine all 6 parameters. Results in part support the conclusions made on $H_{2}O$-type molecules. There appears to be a ""preferred"" strain free bond angle.

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Author Institution: Department of Chemistry, University of Connecticut

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