THE RELATION OF NONADIABATIC ROTATIONAL AND VTBRATIONAL EFFECTS TO ELECTRIC AND MAGNETIC PROPERTIES OF NEUTRAL DIATOMIC MOLECULES AND MOLECULAR IONS

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1997

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Ohio State University

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With several instances we demonstrate that one can derive knowledge about the electric and magnetic properties, specifically the electric dipolar moment and rotational g factor and their dependence on internuclear distance, of both neutral diatomic molecules and molecular ions from purely frequency information, specifically the frequencies and wavenumbers of pure rotational and vibration-rotational transitions in infrared spectra of species consisting of appropriate isotopic variants. We show how such knowledge of electric and magnetic properties from other experiments can serve in analyses of spectra of diatomic molecular species to yield improved values of other molecular properties.

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Author Institution: Department of Chemistry, Oregon State University

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