HELIUM NANODROPLET ISOLATION SPECTROSCOPY USING AN EXTERNAL CAVITY QUANTUM CASCADE LASER

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2009

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Ohio State University

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A mode-hop free tunable external cavity quantum cascade laser (Daylight Solutions) is used to probe the vibrational dynamics of helium solvated H$_{2}$O and NO$_{2}$ monomers and dimers. The demonstrated high output power and mode-hop free tuning of the laser in combination with a multipass cell and bolometric detection allow for high resolution spectroscopy studies of helium solvated molecules between 10 and 5 $\mu$m.

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Author Institution: Department of Chemistry, University of Georgia, Athens, Georgia 30602

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