THE THEORY OF VIBRATIONAL CIRCULAR DICHROISM. I. TECHNIQUES FOR THE CALCULATION OF ROTATIONAL STRENGTHS OF VIBRATIONAL TRANSITIONS

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1979

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Ohio State University

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The calculation of rotational strengths of vibrational transitions requires the evaluation of matrix elements of the electric and magnetic dipole-moment operators and, for this purpose, it is necessary first to solve the normal-coordinate problem. New techniques have been developed for the treatment of redundant coordinates and for the proper inclusion of linear force constants. These techniques are designed for use with a computer and are much simpler than many which have been used previously.

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