LASER PHOTOELECTRON INVESTIGATION OF JET-COOLED 1, 4-DIFLUOROBENZENE.

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1991

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Ohio State University

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Laser photoelectron spectra of jet cooled p-difluorobenzene have been obtained using nanosecond and picosecond ionization pulses. Previously unobserved vibrational levels of the $^{2}B_{2g}$ ion ground state have been recorded. Picosecond pulses have been used with pump - probe multiphoton ionization techniques and laser photoelectron spectroscopy to study the dynamics of the $^{1}B_{2u}$ lowest excited state in p-difluorobenzene. Vibrational levels have been studied including several shown previously to exhibit intramolecular vibrational redistribution (IVR), as well as identifiable Fermi resonance states both above and below the reported IVR threshold.""

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Author Institution: Department of Chemistry, Indiana University

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