ELECTRONIC STRUCTURE OF $ScF_{2}$ AND $TiF_{2}$.

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1969

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Ohio State University

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Abstract

Ab Initio LCAO-MO SCF calculations using a contracted Gaussian basis are reported for several low-lying electronic states of $ScF_{2}$ and $TiF_{2}$. These calculations demonstrate the importance of 4p orbitals for the determination of the equilibrium bond angle and spectra of these species. Various possibilities for the electronic configuration of the ground state are considered and the qualitative features of the spectra are discussed.

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Author Institution: Department of Chemistry, Rice University

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