EXPERIMENTAL DETERMINATION TO LARGE INTERNUCLEAR SEPARATION OF THE '$\Sigma^{+}$ STATE ELECTRIC DIPOLE MOMENT FUNCTION OF CO

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1983

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Ohio State University

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We have experimentally determined the EDMF of CO’s ground electronic state to about the classical turning points of the V=40th level. The $Pade’$ approximant representation of the EDMF is determined via a non-linear least-squares fit which combines numerically obtained vibrational wavefunctions and experimentally determined vibrational band intensities for which $\Delta v=1,2,3$ and 40 for both emission spectra by considering pairs of vibrational transitions from common upper vibrational states and assuming a well defined rotational temperature. These results should be useful in the interpretation of solar infrared spectra.

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Author Institution: NASA Ames Research Center, Astrophysical Experiments Branch; Laboratoire d' Infrarouge, Universite de Paris-Sud. Campus; Institut for Angewandte Physik der, Universitat Bonn Wegel str. 8, 0-5300

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