AB INITO TEST STUDY ON THE VERTICAL EXCITATION ENERGY OF VAN DER WALLS DIMERS

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2000

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Ohio State University

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Abstract

Studies in the framework of the supermolecule approach using high level ab initio methods, of quantum chemistry with different basis sets, constructed to give accurate values for the electric moments and polarizabilities, and supplemented by bond functions placed at the midpoint, will be discussed. Vertical excitation electronic spectra of the diatomic van der Waals $CO- H_{2}$. $CO - He$ and $N_{2} - He$ molecules will be presented and compared with recent experimental results.

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Author Institution: Department of Chemistry, Simon Bolivar University; Department of Chemistry and Biochemistry, Baylor University

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