ULTRASENSITIVE DUAL-BEAM ABSORPTION SPECTROSCOPY, BASED ON WAVELENGTH-MODULATION TECHNIQUE AND LOGARITHMIC NOISE CANCELLING

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1996

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Ohio State University

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Various registration methods for ultrasensitive diode laser based absorption spectroscopy are discussed. The sensitivity of a single-beam wavelength modulation technique is limited by excess laser noise and wavelength-dependent effects in optical system. A dual-beam logarithmic detection allows to reduce excess laser noises but actually shot-noise level is not usually achieved and sensitivity is limited by low-frequency transmittance fluctuations and a flicker noise from atomizer. Simultaneous using a double-beam logarithmic detection and a wavelength-modulation technique allows to minimize a low-frequency noise contribution. Absorbance of $7\times10^{8}$/(Hz)$^{1/2}$ in such a system is demonstrated. Applications to trace measurements of chlorine in glow-discharge atomizer and lithium in graphite tube atomizer are described.

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Author Institution: Insitute of Spectroscopy, Russian Academy of Science

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