HIGH VIBRATIONAL OVERTONES OF SPHERICAL TOP MOLECULES

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1983

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Ohio State University

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We give both a quantum and classical description of the high overtones of spherical top molecules using a generic three dimensional potential surface for the dipole active mode. This potential gives rise to quasi-periodic vibrational ``clusters"" as well as chaotic motion for various anharmonicities and energies. We hope to show the relevant vibrational trajectories in 3-D.

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Author Institution: University of California, Los Alamos National Laboratory, Theoretical Division Los Alamos; Physics Department, Georgia Institute of Technology Atlanta

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