OPTICAL PROPERTIES OF CLUSTERS IN MIXED MOLECULAR CRYSTALS AND APPLICATION TO BENZENE

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1975

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Ohio State University

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A new formalism is given for the optical absorption spectra generated by clusters of guest molecules in substitutionally disordered molecular crystals. The cluster method presented is an extension of the formalism given by Hoshen and $Jortner^{1}$ for calculating the density of states for clusters in mixed molecular crystals. Optical properties are calculated for a one and two dimensional cluster. Results will be compared with experimental data for benzene vibrational excitons.

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$^{1}$J. Hoshen and J. Jortner, J. Chem. Phys. 56, 4138 (1972).""
Author Institution: Department of Chemistry, The University of Michigan

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