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The discovery of \chem{Zn(I)_2}($\eta 5$-\chem{C_5}\chem{Me_5}$)2$ has fundamentally changed the definition of metallocene by introducing dimetallic units to the middle of the classic sandwich complex. Since actinide metallocenes employing COT (COT = [\chem{C_8}\chem{H_8}$]2-$) rings are well known, it occurred to us that uranium dimers may be stabilized by this new bonding motif. Scalar-relativistic density functional theory calculations have been employed to investigate the isomers of [U(\emph{n}$)2$\chem{(COT)_2}$]2\backslash emphn-4$ complexes where \emph{n} = 2 or 3. The IR and NMR vibrational signatures of these complexes is presented to facilitate experimental detection.