ELECTRONIC SPECTROSCOPY OF DIPHENYLAMINE AND ITS SOLVENT CLUSTERS

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1996

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Ohio State University

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The vibrationally resolved electronic spectra of diphenylamine and several isotopically substituted derivatives were recorded using two-photon ionization under supersonic jet expansion conditions. Spectral evidence is consistent with the equivalence of the two phenyl rings which suggests a $C_{2}$ symmetry ground state in which the central nitrogen atom is in a planar configuration. Analysis of the spectrum of diphenylamine clustered with water shows that the solvent has a large influence on the chromophore structure. This contrasts with the observations obtained for diphenylamine clustered with inert gases and nitrogen.

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Author Institution: Department of Chemistry and Center for Photochemical Sciences, Bowling Green State University

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