THE SPECTROSCOPY AND AB INITIO CALCULATION OF THE $C_{3}$ - AR COMPLEX

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2001

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Ohio State University

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The $C_{3}Ar$ van der Waals complex has been produced by photolyzing propargyl bromide at 193 nm in a supersonic molecular beam and probed by the laser-induced fluorescence. The spectroscopy of the ground electronic state of this complex was obtained by the wavelength-resolved emission from the $\tilde{A}$ state. In this preliminary report, the observed vibrational levels of the $C_{3}Ar$ complex were assigned based upon our ab initio results calculated at the MP2/aug-cc-pvtz level.

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Author Institution: ACADEMIA SINICA; INSTITUTE OF ATOMIC AND MOLECULAR SCIENCES, ACADEMIA SINICA

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