ANALYSIS OF ROTATIONAL STRUCTURE IN THE HIGH-RESOLUTION INFRARED SPECTRUM OF CIS,CIS-1,4-DIFLUOROBUTADIENE

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Date

2006

Authors

Craig, Norman C.
Moore, Michael C.
Masiello, Tony

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Ohio State University

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Abstract

We seek an equilibrium structure {\it cis,cis}-1,4-difluorobutadiene. Rotational structure of a C-type band centered at 762.8 cm$^{-1}$ in the high-resolution infrared spectrum (0.0015 cm$^{-1}$) has been analyzed as a first step. A sequence of strong hot bands of the torsional mode (78 cm$^{-1}$) complicate the analysis of this band. Provisional ground state rotational constants are reported. The spectrum of a second C-type band at 328 cm$^{-1}$ may also be analyzable. Ground state rotational constants for a full set of isotopomers are needed. A procedure for synthesizing these species is being explored.

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Author Institution: Department of Chemistry and Biochemistry, Oberlin College, Oberlin, OH 44074; Environmental and Molecular Sciences Laboratory, Pacific Northwest National Laboratory, P.O. Box 999, Mail Stop K8-88, Richland, WA 99352

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