CALCULATION OF DEPOLARIZATION FACTORS FOR SOME HALOGENATED METHANES

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1955

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Ohio State University

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A method has been developed for calculating the depolarization factors of polyatomic molecules. The method is based upon the assumptions made originally by Wolkenstein of the additivity of bond polarzabilities, and some complementary assumption about the dependence of bond polarizabilities on the internal coordinates. Full use is made of the Wilson FG-matrix technique. The method has been tested on some simple substituted methanes. Some modifications in the basic assumption seem to be necessary to give better agreement with experiment.

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Author Institution: Illinois Institute of Technology

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