CALCULATION OF FAR WING LINE BROADENING OF THE SODIUM D LINE INDUCED BY COLLISIONS WITH HYDROGEN ATOMS

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1974

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Ohio State University

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Ab initio MCSCF wavefunctions and energies were calculated at several internuclear distances for the six states of NaH arising from the divided atoms Na($^{2}S$) + H($^{2}S$) and Na($^{2}P$) + H($^{2}S$). The resulting potential curves, and line strengths computed from the wavefunctions, were used in a statistical line shape $calculation^{1}$ to determine the shape of the far wings of the sodium D line broadened by collisions with hydrogen atoms. The most notable feature of the calculated spectrum is a satellite peak at 10 400 {\AA}, whose intensity is $10^{-9}$ that of the central (unperturbed) peak at $5000^{\circ} K$ and a H atom density of $10^{-10}$ $Bohr^{-3}$.

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$^{1}$R.E.M, Hedges, D. L. Drummond, and A. Gallagher, Phys. Rev. A6, 1519 (1972).
Author Institution: Department of Chemistry, University of Chicago; Computer Center, University of Illinois at Chicago Circle

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