LOWER STATE HYPERSURFACES FOR THE $N_{2}O$ SYSTEM

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1974

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Ohio State University

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Reliable theoretical descriptions of the reactions $$\begin {array}{ll} (1) &O(^{1}D) + N_{2} = O(^{3}P) + N_{2}\\ (2) &O(^{3}P) + N_{2}(v = 1) = O(^{3}P) + N_{2} (v = 0)\\ (3) &N_{2}O(^{1}\Sigma^{+}) = N_{2} (^{1}\Sigma^{+}_{g}) + O(^{3}P)\\ \end {array}$$ require the calculation of accurate adiabatic hypersurfaces for the low-lying states of the $N_{2}O$ system. Such surfaces are presently being computed for the lowest $^{1}A^{\prime}$ and $^{3}A^{\prime\prime}$ states. The results and their bearing on Reactions (1)-(3) will be presented and discussed. D. G. Hopper is a NAS-NRC Resident Research Associate. This work is part of a joint project on air triatomics and their positive and negative ions by the groups of T. O. Tiernan, at the Aerospace Research Laboratories (AFSC), USAF, M. Krauss at the National Bureau of Standards, and A. C. Wahl at the Argonne National Laboratories.

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Author Institution: Aerospace Research Laboratories, Wright-Patterson Air Force Base

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