AB INITIO LCAO-MO-SCF CALCULATIONS FOR METHYL NITRATE

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1975

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Ohio State University

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Abstract

The results of ab initio self-consistent field molecular orbital calculations for methyl nitrate will be presented. Two different basis sets have been employed, an STO-3G minimal basis set and a (9s5p/4s2p)(4s/2s) basis set. $Huzinaga’s^{1}$ Gaussian primitives have been contracted using Dunning’s $scheme^{2}$. The calculations will be used to interpret X-ray photoelectron spectroscopic data for the $molecule,^{3}$ and predicted values of some molecular properties will be presented. Preliminary calculations on several excited electronic states will be discussed, with particular attention given to the 3$^{1}$A$^{\prime}$ state.

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$^{1}$ S. Huzinaga, J. Chem, Phys. 42, 1293 (1965). $^{2}$ T. H. Dunning, JR., J. Chem. Phys. 53, 2823 (1970). $^{3}$ G. F. Adams, J. Sharma, and P. DiBona, Manuscript in preparation.""
Author Institution: United States Army Ballistic Research Laboratories, Aberdeen Proving Ground

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