LIF SPECTROSCOPY OF JET-COOLED $CHD_{2}O$

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2002

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Ohio State University

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Abstract

Rotationally resolved Laser-induced Fluorescence measurement is performed on the electronic transition $\tilde{A}^{2} A^{\prime}\leftarrow \tilde{X}^{2} E_{3/2}$ of jet-cooled $CHD_{2}O$ from $2900-3100 cm^{-1}$ in vibrational excitation energy of the $\tilde{A}^{2} A^{\prime}$ state, where ab initio result suggests the fundamental of C-H stretch is located. Resorting to a rotational analysis, eight vibrational bands are recognized and characterized. The vibrational assignments are confirmed by a relative intensity analysis and the symmetries thoughtfully determined in the rotational analysis.

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$^{a}$Novellus Systems, Inc., 2730 Junction Ave., San Jose, CA 95134
Author Institution: Laser Spectroscopy Facility, Department of Chemistry, The Ohio State University; Department of Chemistry of UC Berkeley, Chemical Sciences Division of the Lawrence Berkeley National Laboratory; Laser Spectroscopy Facility, Department of Chemistry, The Ohio State University

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