TRANSIENT FM SPECTROSCOPY FOR DOPPLER MEASUREMENTS OF PHOTOFRAGMENT VELOCITIES AND VECTOR CORRELATIONS

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1996

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Ohio State University

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Doppler-broadened FM line profile of nascent photoproducts have been measured for everal photodissociation systems, We describe methods required for the quantitative analysis of the FM line shapes to give velocity and rotational polarization information. Correlated state distribution and velocity-depended vector correlations can be extracted with relative ease from a set of high-quality line shapes.

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Acknowledgment: This work was carried out under Contact No. DE-AC02-76CH00016 with the U.S. Department of Energy and supported by its Division of Chemical Sciences, Office of Basic Energy Sciences.
Author Institution: Department of Chemistry, Brookhaven National Laboratory

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http://hdl.handle.net/1811/13655

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Abstracts of OSU International Symposium on Molecular Spectroscopy 1990-1999