LASER SPECTROSCOPY OF IRIDIUM MONOBORIDE

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High resolution laser induced fluorescence spectrum of IrB in the spectral region between 545 to 610 nm has been recorded and analyzed. Reacting laser-ablated iridium atoms with 1\% B$_2$H$_6$ seeded in argon produced the IrB molecule. Four vibronic transition bands: (v, 0) with v = 0-3 of an electronic transition system have been observed. Spectra of all four isotopic molecules: $^{191}$Ir$^{10}$B, $^{193}$Ir$^{10}$B, $^{191}$Ir$^{11}$B and $^{193}$Ir$^{11}$B were recorded. Relationship between isotopic molecules confirmed the vibrational quantum number assignment. Preliminary analysis of the rotational lines showed that these vibronic bands are with $\Omega^\prime$ = 2 and $\Omega^{\prime\prime}$ = 3. Partially resolved hyperfine structure conformed to case a$_\beta$ coupling scheme has been observed.

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Author Institution: Department of Chemistry, The University of Hong Kong, Pokfulam Road, Hong Kong

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