SPECTROSCOPY AND HIGH RESOLUTION PHOTOCHEMISTRY OF THE $A^{2}\Pi$ STATE OF THE HCCS RADICAL

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Date

1999

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Ohio State University

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The ``dark'' photodissociating vibronic levels of the $A^{2}\Pi$ state of the radical have been probed in a jet-cooled expansion by the fluorescence depletion spectroscopy (FDS) technique. Over thirty dark levels have been observed within the region of $2000 cm^{-1}$ above the origin. The FDS spectrum compliments previously taken LIF spectrum. Vibronic analysis and fragmentation process will be discussed.

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Author Institution: The Ohio State University, Dept. of Chemistry, Laser Spectroscopy Facility

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