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dc.creatorBartels, N.en_US
dc.creatorSchafer, T.en_US
dc.creatorHuhnert, J.en_US
dc.creatorWodtke, A. M.en_US
dc.creatorField, R. W.en_US
dc.date.accessioned2012-07-09T19:15:33Z
dc.date.available2012-07-09T19:15:33Z
dc.date.issued2012en_US
dc.identifier2012-RG-07en_US
dc.identifier.urihttp://hdl.handle.net/1811/52284
dc.descriptionAuthor Institution: Georg August Universitat Gottingen, Institut fur Physikalische Chemie, Tammanstrasse 6, 37075 Gottingen, Germany; Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, MA 02139, USAen_US
dc.description.abstractFor many experimentalists (especially those, who are not spectroscopists), molecular pertubations are a curse, as they make assignments and analysis of spectral data more difficult. Nevertheless, they can also be a boon! \newline In this talk we will show how a molecular beam of CO in high vibrational states ($v=17,18$) can be prepared by an optical pumping scheme that we call PUMP-PUMP-PERTURB and DUMP (P$^3$D). P$^3$D exploits the loaning, via spin-orbit perturbations, of the large oscillator strength of the 4th positive system, $A ^1 \Pi \leftarrow X ^1 \Sigma ^+$, to the triplet manifold. This allows some nominally spin-forbidden transitions to be exploited in multistep optical pumping schemes. \newline The ability to \textit{state-selectively} prepare CO in high vibrational states opens up new opportunities for molecular beam scattering experiments.en_US
dc.language.isoenen_US
dc.publisherOhio State Universityen_US
dc.titlePRODUCTION OF A BEAM OF HIGHLY VIBRATIONALLY EXCITED CO USING PERTURBATIONSen_US
dc.typeArticleen_US
dc.typeImageen_US
dc.typePresentationen_US


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