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dc.creatorKusaka, R.en_US
dc.creatorEbata, T.en_US
dc.date.accessioned2010-07-12T13:48:10Z
dc.date.available2010-07-12T13:48:10Z
dc.date.issued2010en_US
dc.identifier2010-TB-09en_US
dc.identifier.urihttp://hdl.handle.net/1811/46044
dc.descriptionAuthor Institution: Department of Chemistry, Graduate School of Science, Hiroshima University, Higashi-Hiroshima, 739-8526, Japanen_US
dc.description.abstractThe benzene dimer is excited to the CH stretching vibrational levels by a picosecond IR pulse, and the time evolution of the population of the pumped and redistributed levels are probed by (1+1)REMPI with a picosecond UV pulse. In order to accomplish IR excitation localized in the site of the T-shaped dimer, two dimer isotopomers [(1) Top=C$_6$H$_6$, Stem=C$_6$D$_6$, (2) Top=C$_6$D$_6$, Stem=C$_6$H$_6$] are used. From the time profiles of the pumped and the relaxed levels, the rate constants of intracluster vibrational redistribution (ICVR) at each site and subsequent vibrational predissociation (VP) are discussed.en_US
dc.language.isoenen_US
dc.publisherOhio State Universityen_US
dc.titleVIBRATIONAL ENERGY RELAXATION OF BENZENE DIMER STUDIED BY PICOSECOND TIME-RESOLVED INFRARED-ULTRAVIOLET PUMP-PROBE SPECTROSCOPYen_US
dc.typeArticleen_US
dc.typeImageen_US
dc.typePresentationen_US


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