A NOVEL TWO-PHOTON ABSORPTION LASER SYSTEM AND EXCITATION SPECTRA OF GASEOUS MOLECULES

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1977

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Ohio State University

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A novel two-photon absorption (TPA) laser system in cw single-mode operation vas built to demonstrate the feasibility of observing two-photon excitation spectra of gaseous molecules. A commercial cw dye laser was modified to perform the intracavity TPA work. The two-photon excitation spectrum of naphthalene (0.07 Torr) with superb signal-to-noise ratios is presented to illustrate the applicability of this new technique.

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Author Institution: Ames Laboratory - ERDA and Department of Chemistry, Iowa State University

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