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C$_{60}^+$ AND C$_{60}^-$ IN NEON AND ARGON MATRICES

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/52191

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Title: C$_{60}^+$ AND C$_{60}^-$ IN NEON AND ARGON MATRICES
Creators: Kern, Bastian; Strelnikov, Dmitry; Weis, Patrik; Bottcher, Artur; Kappes, Manfred M.
Issue Date: 2012
Abstract: Mass-selected C$_{60}$ anions have been deposited in noble gas matrices (Ne,Ar) kept at ~6K. The vibronic properties of the species (C$_{60}^+$, C$_{60}^0$, C$_{60}^-$) were determined by NIR and MID-IR absorption spectroscopy. By co-depositing electrons without the addition of electron scavengers or donors to the host matrix, we were able to vary the C$_{60}^+$/C$_{60}^-$ ratio. By changing the C$_{60}^+$/C$_{60}^-$ ratio, previously known vibrational data of the C$_{60}^+$ and C$_{60}^-$ species could be confirmed and also extended further. DFT calculations performed on isolated C$_{60}^+$ and C$_{60}^-$ ions support the experimental assignment.
URI: http://hdl.handle.net/1811/52191
Other Identifiers: 2012-MJ-08
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