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DEVELOPMENT OF BROAD RANGE SCAN CAPABILITIES WITH JET COOLED CAVITY RINGDOWN SPECTROSCOPY

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/49449

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Title: DEVELOPMENT OF BROAD RANGE SCAN CAPABILITIES WITH JET COOLED CAVITY RINGDOWN SPECTROSCOPY
Creators: Codd, Terrance J.; Chen, Ming-Wei; Miller, Terry A.
Issue Date: 2011
Abstract: We have developed a technique for obtaining broad scans, $>$100 cm$^{-1}$, for jet cooled cavity ringdown spectroscopy $($CRDS$)$ spectra. Previously the scans of the jet cooled, CRDS apparatus were limited to $<$10 cm$^{-1}$ due to the use of a narrow linewidth radiation source. However, by coupling our jet cooled, CRDS apparatus with a moderate resolution~($\simeq$ 0.05 cm$^{-1}$) dye laser we are able to greatly increase our rate of data acquisition thereby gaining the capability to perform broad spectral surveys of jet cooled molecules. As a test of the capabilities of the technique we have scanned the $\tilde{A}$--$\tilde{X}$ transition of NO$_3$ previously reported by Deev \emph{et al.} at room temperature. We believe that this will be a very useful technique to search for transitions of cold molecules whose frequencies are not well known and which later can be studied using high resolution methods.
URI: http://hdl.handle.net/1811/49449
Other Identifiers: 2011-TD-06
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