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INFRARED LASER SPECTROSCOPY OF (HCl)$_{m}$ ??( H$_{2}$O)??$_{n}$ CLUSTERS IN HELIUM NANODROPLETS

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dc.creator Flynn, S. D. en_US
dc.creator Morrison, A. M. en_US
dc.creator Liang, T. en_US
dc.creator Douberly, G. E. en_US
dc.date.accessioned 2010-07-12T14:34:54Z
dc.date.available 2010-07-12T14:34:54Z
dc.date.issued 2010 en_US
dc.identifier 2010-FB-08 en_US
dc.identifier.uri http://hdl.handle.net/1811/46452
dc.description Author Institution: Department of Chemistry, University of Georgia, Athens, GA 30602 en_US
dc.description.abstract Small hydrogen chloride-water clusters are of great theoretical and experimental interest, with much recent attention focusing on HCl charge dissociation in small water clusters. We have employed Helium Nanodroplet Isolation techniques to definitively assign bands in the 2570-2900 cm$^{-1}$ range to specific (HCl)$_{m}$ ??(H$_{2}$O)??$_{n}$ clusters. Vibrational Transition Moment Angle (VTMA) analysis, dipole moment measurements, optically selected mass spectrometry (OSMS), pick up cell pressure dependence studies and \textit{ab initio} calculations are all used together to arrive at the assignments. We will discuss these new assignments in the context of the vibrational dynamics of the H$_{3}$O$^{+}$(H$_{2}$O)$_{n>3}$Cl$^{-}$ charge separated species. en_US
dc.language.iso en en_US
dc.title INFRARED LASER SPECTROSCOPY OF (HCl)$_{m}$ ??( H$_{2}$O)??$_{n}$ CLUSTERS IN HELIUM NANODROPLETS en_US
dc.type Article en_US
dc.type Image en_US
dc.type Presentation en_US