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DETECTION OF THE MAGNETIC DIPOLE-ALLOWED ORIGIN BAND OF THE $\widetilde{A}$$\leftarrow$$\widetilde{X}$ TRANSITION OF THE NITRATE RADICAL NO$_3$

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/38344

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Title: DETECTION OF THE MAGNETIC DIPOLE-ALLOWED ORIGIN BAND OF THE $\widetilde{A}$$\leftarrow$$\widetilde{X}$ TRANSITION OF THE NITRATE RADICAL NO$_3$
Creators: Takematsu, Kana; Eddingsaas, Nathan; Okumura, Mitchio; Stanton, John
Issue Date: 2009
Abstract: Despite its simplicity and atmospheric significance, the lowest electronic states of NO$_3$ remain poorly understood. The $\widetilde{A}$$^2$E$^{\prime \prime}$ state is Jahn-Teller (JT) active and is pseudo-JT coupled to the ground $\widetilde{X}$$^2$A$_2$$^{\prime}$ and excited $\widetilde{B}$$^2$E$^{\prime \prime}$ states. While the band origin 0$^{0}_{0}$ of the $\widetilde{A}$$\leftarrow$$\widetilde{X}$ transition is purely electric forbidden, the cavity ringdown spectrum of the vibronically-allowed $\widetilde{A}$$\leftarrow$$\widetilde{X}$ bands has shown rotationally-resolvable structures. We have detected the magnetic dipole-allowed origin ($\sim$7060 cm$^{-1}$) via CRD spectroscopy. Analysis of the band contour along with its implications of the JT/Pseudo-JT couplings in the dark $\widetilde{A}$ state of NO$_3$ will be discussed.
URI: http://hdl.handle.net/1811/38344
Other Identifiers: 2009-RD-02
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