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THE ELECTRONIC SPECTRUM AND RENNER-TELLER ANALYSIS OF THE C$_2$P FREE RADICAL

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/33253

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Title: THE ELECTRONIC SPECTRUM AND RENNER-TELLER ANALYSIS OF THE C$_2$P FREE RADICAL
Creators: Sunahori, Fumie X.; Wei, Jie; Clouthier, Dennis J.
Issue Date: 2008
Abstract: Subsequent to our spectroscopic detection of the C$_2$X (X = P, As) free radicals,} \underline {\textbf{129}} (9600), 2007.} we have studied the electronic spectrum of the jet-cooled $^2\Delta$${_i}$ - $^2\Pi$${_r}$ system of the C$_2$P free radical in the 490-630 nm region. High resolution spectra of the two spin-components of the $0_0^0$ band of $^{12}$C$_2$P have been recorded, and the rotational and spin-orbit coupling constants have been determined for both electronic states. Evidence of the Renner-Teller effect has been observed in both the $^2\Pi$${_r}$ and $^2\Delta$${_i}$ states, and the vibrational structure has been assigned and fitted to a Renner-Teller hamiltonian for $^{12}$C$_2$P and $^{13}$C$_2$P. The molecular parameters predicted by density functionl theory are in good agreement with the derived experimental values and provide validation for the spectroscopic assignments. The molecular structure of C$_2$P in the ground and excited state will be discussed.
URI: http://hdl.handle.net/1811/33253
Other Identifiers: 2008-WI-04
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