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THE X $\leftarrow$ A SEP SPECTRA OF JET-COOLED THIOPHOSGENE

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/31310

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Title: THE X $\leftarrow$ A SEP SPECTRA OF JET-COOLED THIOPHOSGENE
Creators: Chowdary, Praveen D.; Strickler, Brent; Lee, Sandra; Gruebele, M.
Issue Date: 2007
Abstract: \noindent The \ {X} $\leftarrow$ \ {A} stimulated emission pumping of SCCl$_2$ made over 100 new vibrational transitions accessible from 7000 -- 8000 cm$^{-1}$ above the \ {X} state zero point energy.} We report anharmonic constants that fit all the 482 currently assigned vibrational energy levels. A spectral autocorrelation analysis shows that the onset of free energy flow has not been reached at 8000 cm$^{-1}$, in accordance with higher energy \ {B} state SEP data and a theoretical analysis. The available experimental data and computational results are both compatible with less fragmentation among the observable interior states of SCCl$_2$.
URI: http://hdl.handle.net/1811/31310
Other Identifiers: 2007-WH-06
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