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HIGH-RESOLUTION LASER-INDUCED FLUORESCENCE (LIF) SPECTROSCOPY OF THE DEUTERATED ISOTOPOMERS OF THE METHOXY RADICAL

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/30741

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Title: HIGH-RESOLUTION LASER-INDUCED FLUORESCENCE (LIF) SPECTROSCOPY OF THE DEUTERATED ISOTOPOMERS OF THE METHOXY RADICAL
Creators: Liu, Jinjun; Yi, John T.; Miller, Terry A.
Issue Date: 2006
Abstract: \maketitle Our high-resolution laser-induced fluorescence (LIF)spectroscopy apparatus has been improved to study the deuterated isotopomers of the methoxy radical under jet-cooled conditions (T$\sim$2K). Doppler-free absorption spectra of iodine molecule were recorded simultaneously for absolute calibration,}, Japan Society for the Promotion of Science, (2002).} while relative calibration was done using the fringes of a new etalon. The spectral resolution (FWHM) for methoxy was limited to $\sim$300MHz by residual Doppler broadening and unresolved hyperfine structure. The center of spectral lines could be determined to $\sim$1/5 the FWHM with a comparable absolute accuracy (1$\sigma$$\sim$50MHz). The 3$_0 ^2$ and (6$^{\prime}$)$_0 ^1$ bands of the $\tilde{A}^{2}$A$_1$--$\tilde{X}^{2}$E$_{3/2}$ transition for CHD$_{2}$O and CH$_{2}$DO have been recorded, as well as the 3$_0 ^2$ and 6$_0^1$ bands for CH$_{3}$O and CD$_{3}$O. Rotational and fine structure for all bands has been resolved and assigned. Details of the analyses will be presented in the following talks.
URI: http://hdl.handle.net/1811/30741
Other Identifiers: 2006-TJ-04
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