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STARK EFFECT IN X$_2$Y$_4$ MOLECULES: APPLICATION TO ETHYLENE

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/30375

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Title: STARK EFFECT IN X$_2$Y$_4$ MOLECULES: APPLICATION TO ETHYLENE
Creators: Rotger, M.; Raballand, W.; Boudon, V.; Loete, M.; Breidung, Jurgen; Thiel, Walter
Issue Date: 2005
Abstract: We present a development of the dipole moment and polarizability operators of X$_2$Y$_4$ molecules, using a tensorial formalism} {\bf 217}, 239-248, (2003)}$^,$}, accepted, (2005).} analogous to the one developed for tetrahedral and octahedral molecules} {\bf 228}, 620-634, (2004).}. These operators are involved in the calculation of the intensities of rovibrational transitions as well as in the calculation of the Stark effect. Expressions for the matrix elements are derived. A model for the study of the Stark effect in isolated bands of such molecules is proposed and has been used to predict the Stark spectra of the $\nu_{12}$ band of ethylene. Values of the polarizability coefficients have been calculated using {\em ab initio} methods.
URI: http://hdl.handle.net/1811/30375
Other Identifiers: 2005-MJ-12
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