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CaF: ALL SPECTRA AND ALL DYNAMICS

Please use this identifier to cite or link to this item: http://hdl.handle.net/1811/46084

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Title: CaF: ALL SPECTRA AND ALL DYNAMICS
Creators: Field, R. W.; Kay, J. J.; Coy, S. L.; Petrovic, V. S.; Altunata, S. N.; Wong, B. M.; Jungen, Ch.
Issue Date: 2010
Publisher: Ohio State University
Abstract: More than 1,000 CaF rovibronic levels, spanning the range $n^{*}=5,\ v=0\ (42,500 $ cm$^{-1}) $ to $ n^{*}=20,\ v=1\ (47,500 $ cm$^{-1})$, and sampling $\ell=0(s)-5(h)$ are fitted to a quantum defect model. This model consists of two currently separate pieces: the core-penetrating $s,\ p,\ d,\ f$ series are fitted to the elements of an internuclear distance $(R)$ and energy $(E)$ dependent quantum defect matrix, $\mu(R,E)$; the core-nonpenetrating series are described by multipole $(\mu,\ Q,\ O)$ moments and polarizabilities $(\alpha,\ \gamma)$. The values of the fitted parameters agree well with $ab\ initio$ computed values. Although the fitted parameters permit calculation of all spectra and all dynamics of CaF, the physical meanings of the parameters remain obscure.
URI: http://hdl.handle.net/1811/46084
Other Identifiers: 2010-TG-06
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